Past three or four weeks I've jumped in and have been trying to learn Engrosser's script (Copperplate, Zanerian, etc.). Some really great resources are the IAMPETH website, Dr. Joe Vitolo's articles, a terrific DVD by Wm.Lilly, and a few books such as Mastering Copperplate Calligraphy.
I'm using HP 24lb laser paper, an oblique pen holder, either Higgins Eternal or McCaffrey's (iron gall) ink, and a variety of pointed pens, my favorites being Hunt 101, Zebra G, Hiro 40 and Hunt 108 crowquill.
Here's where I'm at after these few weeks (a practice sample I did this morning, took about 20-30 minutes) - please critique ruthlessly and offer any suggestions you might have. Truly fun to approach this beautiful form.
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